In forty plus years of performance and teaching, I've found that Blazhevich, Kopprasch and Bordogni are some of the best method books for tubists of all levels. In each, you'll find plenty of examples to challenge and refine your articulation, phrasing, knowledge of keys and interpretation. I still use my dog-eared copies to this day whenever I need to get the rust out of my chops. When you can play the Blazhevich 70 Studies all the way through, there will never be another key that will give you pause.
Other sheet music offered here are resources that I've found useful for various levels of student abilities. All are well worth the investment and will be part of your library for years to come.
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